Fine structure of K<SUB>3</SUB>C<SUB>60</SUB> photoionization cross-section oscillations

LI Hong-Nian; YING Li-Jian; NI Jing-Fu; LI Gang; WANG Peng; KURASH Ibrahim; QIAN Hai-Jie

doi:10.1088/1674-1137/33/11/012

Chinese Physics C> 2009, Vol. 33> Issue(11) : 991-995 DOI: 10.1088/1674-1137/33/11/012

Fine structure of K₃C₆₀ photoionization cross-section oscillations

Abstract
HTML
Reference
Related

PDF

Abstract：
The synchrotron radiation angle-resolved photoemission data of K₃C₆₀ single crystal film are analyzed, aiming at the photoionization cross-sections of the LUMO, HOMO and HOMO-1 bands in low photon energy region (14.5—27.5 eV). Many fine structures of the HOMO/HOMO-1 intensity ratios are observed, which support the general validity of a quantum chemistry model. However, the experimental data and the theoretical results have some disagreement in the energy positions and magnitudes of the fine structures, and the disagreement is more outstanding than the case of pure C₆₀. So the photoemission data of K₃C₆₀ afford valuable experimental reference to further theoretical developments. The LUMO cross-section data, which cannot be discussed with the quantum chemistry description due to strong solid state effects, are also reported for further studies.

References

[1]

. Benning P J, Poirier D M, Troullier N et al. Phys. Rev. B,1991, 44: 1962-19652. Liebsch T, Plotzke O, Heiser F et al. Phys. Rev. A, 1995,52: 457-4643. LI H N, NI J F, YING L J et al. J. Phys.: Condens. Matter,2007, 19: 4362234. Venuti M, Stener M, Alti G De et al. J. Chem. Phys., 1999,111: 4589-45975. Decleva P, Furlan S, Fronzoni G et al. Chem. Phys. Lett.,2001, 348: 363-3676. Decleva P, Fronzoni G, Stener M et al. Phys. Rev. Lett.,2005, 95: 2634017. XU Y B, TAN M Q, Becker U. Phys. Rev. Lett., 1996, 76:3538-35418. Rudel A, Hentges R, Becker U et al. Phys. Rev. Lett., 2002,89: 1255039. Frank O, Rost J M. Chem. Phys. Lett., 1997, 271: 367-37110. Hasegawa S, Miyamae T, Yakushi K et al. Phys. Rev. B,1998, 58: 4927-493311. HE S L, LI H N, WANG X X et al. Phys. Rev. B, 2005,71: 08540412. Hunt M R C, Pichler T, #352;iller L et al. Phys. Rev. B, 2002,66: 19340413. LI H N, XU Y B, BAO S N et al. Phys. Rev. B, 2000, 61:13256-1326014. TAN M Q, XU B, LI H N et al. J. Cryst. Growth, 1997,182: 375-37815. Bertsch G F, Bulgac A, Tomanek D et al. Phys. Rev. Lett.,1991, 67: 2690-269316. Panaccione G, Altarelli M, Fondacaro A et al. Phys. Rev.Lett., 2006, 97: 11640117. Nasu K, Yamazaki M, Tomita N et al. J. Electron Spectrosc.Relat. Phenom., 2004, 136: 49-56

[1]	Hong-Dou Jin;Li-Peng Zhou;Bing-Xin Zhang;Hai-Ming Hu . A discussion on vacuum polarization correction to the cross-section of ${e^+e^-\to\gamma^\ast/\psi\to\mu^+\mu^-}$. Chinese Physics C, 2019, df87c41e-622f-49a7-b081-5c584df157aa(11): 13104-.
[2]	Guo-Zhu He , Bin Shi , Ming He , Zhen-Yu Li , Shi-Long Liu , Xiong-Jun Chen , Xi-Chao Ruan , Qi-Wei Zhang , Qi-Wen Fan , Heng Li , Shao-Yong Wu , Shan Jiang , Zu-Ying Zhou . Cross-section measurement for the ⁹³Nb(n, 2n)^92gNb reaction at the neutron energy of 14.6 MeV by the AMS method. Chinese Physics C, 2018, 42(7): 074002. doi: 10.1088/1674-1137/42/7/074002
[3]	M. Ablikim , et al . Measurement of the integrated Luminosities of cross-section scan data samples around the ψ(3770) mass region. Chinese Physics C, 2018, 42(6): 063001. doi: 10.1088/1674-1137/42/6/063001
[4]	Rajnikant Makwana , S. Mukherjee , Jian-Song Wang , Zhi-Qiang Chen . New empirical formula for (γ, n) reaction cross section near GDR peak for elements with Z≥60. Chinese Physics C, 2017, 41(4): 044105. doi: 10.1088/1674-1137/41/4/044105
[5]	S. A. Alavi , V. Dehghani . Alpha-induced reaction cross-section for Sm, U, Np targets: influence of hexadecapole deformation and deformed surface diffuseness. Chinese Physics C, 2017, 41(6): 064104. doi: 10.1088/1674-1137/41/6/064104
[6]	S. A. Seyyedi , H. Golnarkar . Nuclear matter incompressibility effect on the cross-section offusion reactions with a weakly bound projectile. Chinese Physics C, 2015, 39(8): 084103. doi: 10.1088/1674-1137/39/8/084103
[7]	YE Qing , CHEN Xing , ZHOU Jing , ZHAO Hai-Feng , CHU Wang-Sheng , ZHENG Xu-Sheng , WU Zi-Yu . Local hydrated structure of an Fe²⁺/Fe³⁺ aqueous solution: an investigation using a combination of molecular dynamics and X-ray absorption fine structure methods. Chinese Physics C, 2013, 37(3): 038003. doi: 10.1088/1674-1137/37/3/038003
[8]	ZHOU Feng-Qun , TIAN Ming-Li , SONG Yue-Li , LAN Chang-Lin , KONG Xiang-Zhong . Activation cross-section measurement of a sort of nuclide produced with a target including two isotopes. Chinese Physics C, 2013, 37(8): 084002. doi: 10.1088/1674-1137/37/8/084002
[9]	GUO Shuang , HU Zhen , QIAN Si-Jin , YANG Zong-Chang , LIU Lie . Feasibility study on cross-section measurement of Υ(1S)→μ⁺μ^－ by using early CMS data. Chinese Physics C, 2010, 34(8): 1037-1044. doi: 10.1088/1674-1137/34/8/001
[10]	FANG Kai-Hong , XU Xiao-San , LAN Chang-Lin , YUAN Ji-Long , KONG Xiang-Zhong . Cross-section measurement for Ni(n,x)^58(m+g)Co,Ni(n, x)^60mCo, Ni(n,x)⁶¹Co and Ni(n,x)^62mCo reactions induced by neutrons around 14MeV. Chinese Physics C, 2008, 32(4): 251-253. doi: 10.1088/1674-1137/32/4/002
[11]	YANG Wei-Fan , DING Hua-Jie , YUAN Shuang-Gui , XU Yan-Bing , ZHANG Sheng-Dong , LU Xi-Ting . Production cross-section of ²³⁰Ra in the reaction of 60 MeV/u ¹⁸O ions with ²³⁸U. Chinese Physics C, 2008, 32(S2): 56-58.
[12]	YANG Wei-Fan , XU Yan-Bing , DING Hua-Jie , YUAN Shuang-Gui . Production Cross-Section of ²³⁶Th in the Interaction of ²³⁸U with 60MeV/u ¹⁸O Ions. Chinese Physics C, 2006, 30(S2): 189-191.
[13]	XU Ya-Bo , LI Hong-Nian , BAO Shi-Ning , LI Hai-Yang , QIAN Hai-Jie , LIU Feng-Qin , Kurash Ibrahim , JIA Jin-Feng , XUE Qi-Kun . Synchrotron Radiation Angle-Resolved Photoemission Study of the Orientational Phase Transition for K₃C₆₀. Chinese Physics C, 2001, 25(S1): 33-38.
[14]	YANG Min , CHEN GuoMing , YANG HaiJun , XIONG ZhaoHua , LU YuSheng , CHEN HeSheng . Measurement of the Cross-Section of Single W Boson Production and the Anomalous Couplings on L3 Experiment. Chinese Physics C, 2000, 24(12): 1073-1080.
[15]	Wang Qi , Lu Jun , Xu Hushan , Li Songlin , Zhu Yongtai , Yin Xu , Fan Enjie , Zhang Yuhu , Li Zhichang , Zhao Kui , Lu Xiuqin , Hu Xiaoqing . Cross-Section Fluctuation of the Isotope Projectile-like Fragments in the Dissipative Reaction ¹⁹F+⁵¹V. Chinese Physics C, 1996, 20(S2): 113-120.
[16]	Wang Jicheng , Zhang Li , Guo guanghui , Zhao Jinhua , Zheng Jiwen . Cross-section Measurement of Neutron-Rich Hg Nuclides in Reaction of 28 MeV/u ¹⁸O with Thick Natural Lead Target. Chinese Physics C, 1995, 19(S3): 241-246.
[17]	Li Tingyan , Shi Zhaomin , Lu Hanlin , Zhao Wenrong , Yu Weixiang , Yuan Xialin . Cross Section Measurement and Evaluation for ⁵⁸Ni(n,p),⁶⁰Ni(n,p), ⁶²Ni(n,α) and ⁵⁴Fe(n,p) Reactions. Chinese Physics C, 1991, 15(S4): 341-351.
[18]	Wang Yongchang , Yuan Junqian , Ren Zhongliang , Wang Huamin , Yang Jingkang , Shui Yongqing , Xiang Sicang . Cross Section Measurement of the ⁶³Cu(n,α)⁶⁰Co Reaction. Chinese Physics C, 1991, 15(S1): 73-77.
[19]	WANG Yong-Chang , REN Zhong-Liang , YUAN Jun-Qian , YANG Jing-Kang , XIANG Si-Cang . THE CROSS SECTION MEASUREMENT FOR THE ⁶⁰Ni(n,p)⁶⁰Co REACTION. Chinese Physics C, 1990, 14(10): 923-926.
[20]	SONG Xiao-Tong , DAI You-Shan . THE COULOMB DISINTEGRATION CROSS-SECTION AND DECAY RATE OF THE SPIN (0－3/2) ELECTROMAGNETIC BOUND SYSTEM. Chinese Physics C, 1987, 11(1): 24-31.

Access

Get Citation

LI Hong-Nian, YING Li-Jian, NI Jing-Fu, LI Gang, WANG Peng, KURASH Ibrahim, QIAN Hai-Jie and Fine structure of K₃C₆₀ photoionization cross-section oscillations[J]. Chinese Physics C, 2009, 33(11): 991-995. doi: 10.1088/1674-1137/33/11/012

RIS(for EndNote,Reference Manager,ProCite)

BibTex

Txt

Milestone

Received: 2008-12-18
Revised: 2009-03-31

Article Metric

Article Views(2704)
PDF Downloads(532)
Cited by(0)

Policy on re-use

To reuse of subscription content published by CPC, the users need to request permission from CPC, unless the content was published under an Open Access license which automatically permits that type of reuse.

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Fine structure of K₃C₆₀ photoionization cross-section oscillations

Corresponding author: LI Hong-Nian,

Received Date: 2008-12-18

Accepted Date: 2009-03-31

Available Online: 2009-11-05

Abstract:

The synchrotron radiation angle-resolved photoemission data of K₃C₆₀ single crystal film are analyzed, aiming at the photoionization cross-sections of the LUMO, HOMO and HOMO-1 bands in low photon energy region (14.5—27.5 eV). Many fine structures of the HOMO/HOMO-1 intensity ratios are observed, which support the general validity of a quantum chemistry model. However, the experimental data and the theoretical results have some disagreement in the energy positions and magnitudes of the fine structures, and the disagreement is more outstanding than the case of pure C₆₀. So the photoemission data of K₃C₆₀ afford valuable experimental reference to further theoretical developments. The LUMO cross-section data, which cannot be discussed with the quantum chemistry description due to strong solid state effects, are also reported for further studies.

HTML

Reference (1)

Fine structure of K₃C₆₀ photoionization cross-section oscillations

Abstract：

References

Access

Article Metrics

Metrics

通讯作者: 陈斌, bchen63@163.com

Email This Article

Fine structure of K₃C₆₀ photoionization cross-section oscillations

Corresponding author: LI Hong-Nian,

HTML

目录

Fine structure of K3C60 photoionization cross-section oscillations

Abstract：

References

Access

Article Metrics

Metrics

通讯作者: 陈斌, bchen63@163.com

Email This Article

Fine structure of K3C60 photoionization cross-section oscillations

Corresponding author: LI Hong-Nian,

HTML

目录

Fine structure of K₃C₆₀ photoionization cross-section oscillations

Fine structure of K₃C₆₀ photoionization cross-section oscillations